Strong coupling of emitters to single plasmonic nanoparticles: Exciton-induced transparency and Rabi splitting

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dc.contributor.authorPelton, Matthew
dc.contributor.authorStorm, S. David
dc.contributor.authorLeng, Haixu
dc.date.accessioned2022-07-11T21:10:24Z
dc.date.available2022-07-11T21:10:24Z
dc.date.issued2019-07-22
dc.description.abstractStrong coupling between plasmons in metal nanoparticles and single excitons in molecules or semiconductor nanomaterials has recently attracted considerable experimental effort for potential applications in quantum-mechanical and classical optical information processing and for fundamental studies of light–matter interaction. Here, we review the theory behind strong plasmon–exciton coupling and provide analytical expressions that can be used for fitting experimental data, particularly the commonly measured scattering spectra. We re-analyze published data using these expressions, providing a uniform method for evaluating and quantifying claims of strong coupling that avoids ambiguities in distinguishing between Rabi splitting and exciton-induced transparency (or Fano-like interference between plasmons and excitons).en_US
dc.description.sponsorshipWe thank Molly May for assistance with figures. M.P. thanks Maxim Sukharev and David Masiello for helpful discussions. This work was supported in part by the National Institute of Standards and Technology under award number 70NANB18H282.en_US
dc.description.urihttps://pubs.rsc.org/en/content/articlelanding/2019/nr/c9nr05044ben_US
dc.format.extent11 pagesen_US
dc.genrejournal articlesen_US
dc.genrepreprintsen_US
dc.identifierdoi:10.13016/m2qoiq-hctm
dc.identifier.citationPelton, Matthew, S. David Storm and Haixu Leng. “Strong coupling of emitters to single plasmonic nanoparticles: Exciton-induced transparency and Rabi splitting.” Nanoscale 11 (2019):14540-14552. http://dx.doi.org/10.1039/C9NR05044Ben_US
dc.identifier.urihttps://doi.org/10.1039/C9NR05044B
dc.identifier.urihttp://hdl.handle.net/11603/25132
dc.language.isoen_USen_US
dc.publisherRoyal Society of Chemistryen_US
dc.relation.isAvailableAtThe University of Maryland, Baltimore County (UMBC)
dc.relation.ispartofUMBC Physics Department Collection
dc.relation.ispartofUMBC Faculty Collection
dc.relation.ispartofUMBC Student Collection
dc.rightsThis item is likely protected under Title 17 of the U.S. Copyright Law. Unless on a Creative Commons license, for uses protected by Copyright Law, contact the copyright holder or the author.en_US
dc.titleStrong coupling of emitters to single plasmonic nanoparticles: Exciton-induced transparency and Rabi splittingen_US
dc.typeTexten_US
dcterms.creatorhttps://orcid.org/0000-0002-6370-8765en_US
dcterms.creatorhttps://orcid.org/0000-0002-1480-6959en_US

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