Quantum-dot-induced transparency in a nanoscale plasmonic resonator

dc.contributor.authorWu, Xiaohua
dc.contributor.authorGray, Stephen K.
dc.contributor.authorPelton, Matthew
dc.date.accessioned2023-08-14T19:12:33Z
dc.date.available2023-08-14T19:12:33Z
dc.date.issued2010-10-26
dc.description.abstractWe investigate the near-field optical coupling between a single semiconductor nanocrystal (quantum dot) and a nanometer-scale plasmonic metal resonator using rigorous electrodynamic simulations. Our calculations show that the quantum dot produces a dip in both the extinction and scattering spectra of the surface-plasmon resonator, with a particularly strong change for the scattering spectrum. A phenomenological coupled-oscillator model is used to fit the calculation results and provide physical insight, revealing the roles of Fano interference and hybridization. The results indicate that it is possible to achieve nearly complete transparency as well as enter the strong-coupling regime for a single quantum dot in the near field of a metal nanostructure.en_US
dc.description.sponsorshipWork at the Center for Nanoscale Materials was supported by the U. S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. We thank Jason M. Montgomery, Tae-Woo Lee, and Lina Cao for help with FDTD programming. The submitted manuscript has been created by UChicago Argonne, LLC, Operator of Argonne National Laboratory (“Argonne”). Argonne, a U.S. Department of Energy Office of Science laboratory, is operated under Contract No. DE-AC02-06CH11357. The U.S. Government retains for itself, and others acting on its behalf, a paid-up nonexclusive, irrevocable worldwide license in said article to reproduce, prepare derivative works, distribute copies to the public, and perform publicly and display publicly, by or on behalf of the Government.en_US
dc.description.urihttps://opg.optica.org/oe/fulltext.cfm?uri=oe-18-23-23633&id=206876en_US
dc.format.extent13 pagesen_US
dc.genrejournal articlesen_US
dc.identifierdoi:10.13016/m2zq1t-opar
dc.identifier.citationWu, Xiaohua, Stephen K. Gray, and Matthew Pelton. “Quantum-Dot-Induced Transparency in a Nanoscale Plasmonic Resonator.” Optics Express 18, no. 23 (November 8, 2010): 23633–45. https://doi.org/10.1364/OE.18.023633.en_US
dc.identifier.urihttps://doi.org/10.1364/OE.18.023633
dc.identifier.urihttp://hdl.handle.net/11603/29208
dc.language.isoen_USen_US
dc.publisherOpticaen_US
dc.relation.isAvailableAtThe University of Maryland, Baltimore County (UMBC)
dc.relation.ispartofUMBC Physics Department Collection
dc.rightsThis work was written as part of one of the author's official duties as an Employee of the United States Government and is therefore a work of the United States Government. In accordance with 17 U.S.C. 105, no copyright protection is available for such works under U.S. Law.en_US
dc.rightsPublic Domain Mark 1.0*
dc.rights.urihttp://creativecommons.org/publicdomain/mark/1.0/*
dc.titleQuantum-dot-induced transparency in a nanoscale plasmonic resonatoren_US
dc.typeTexten_US
dcterms.creatorhttps://orcid.org/0000-0002-6370-8765en_US

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