Ultrastrong coupling of polar phonons and effective epsilon-near-zero modes in coaxial nanocavities

dc.contributor.authorYoo, Daehan
dc.contributor.authorLeon-Perez, Fernando de
dc.contributor.authorLee, In-Ho
dc.contributor.authorMohr, Daniel A.
dc.contributor.authorPelton, Matthew
dc.contributor.authorRaschke, Markus B.
dc.contributor.authorCaldwell, Joshua D.
dc.contributor.authorMartın-Moreno, Luis
dc.contributor.authorOh, Sang-Hyun
dc.date.accessioned2020-04-14T16:50:34Z
dc.date.available2020-04-14T16:50:34Z
dc.date.issued2020-02-29
dc.description.abstractUltrastrong coupling (USC), where the light-matter coupling strength is comparable to the resonance frequency of the uncoupled bare system, presents new frontiers in nanophotonics. However, it has remained notoriously difficult to achieve experimentally. Here we demonstrate USC between polar phonons and mid-infrared (MIR) light in coaxial nanocavities. We achieved a level splitting of strongly coupled polaritons of 50% of the resonant frequency, enabled by the effective epsilon-near-zero (ENZ) responses in the MIR of the SiO2-filled coaxial nanocavities. We theoretically describe this unusually large level splitting as USC using a 2x2 matrix form derived from the coupling of polar phonon lattice and Maxwell's equations. Our wafer-scale coaxial ENZ nanocavity platform offers new routes to explore the physics of vibrational USC within polaritonic systems and harness a broad range of resonant transitions in the MIR regime.en_US
dc.description.urihttps://arxiv.org/abs/2003.00136en_US
dc.format.extent32 pagesen_US
dc.genrejournal article preprintsen_US
dc.identifierdoi:10.13016/m2etho-fpd7
dc.identifier.citationYoo, Daehan; Leon-Perez, Fernando de; Lee, In-Ho; Mohr, Daniel A.; Pelton, Matthew; Raschke, Markus B.; Caldwell, Joshua D.; Martın-Moreno, Luis; Oh, Sang-Hyun; Ultrastrong coupling of polar phonons and effective epsilon-near-zero modes in coaxial nanocavities; Optics (2020); https://arxiv.org/abs/2003.00136en_US
dc.identifier.urihttp://hdl.handle.net/11603/18038
dc.language.isoen_USen_US
dc.relation.isAvailableAtThe University of Maryland, Baltimore County (UMBC)
dc.relation.ispartofUMBC Physics Department Collection
dc.relation.ispartofUMBC Faculty Collection
dc.rightsThis item is likely protected under Title 17 of the U.S. Copyright Law. Unless on a Creative Commons license, for uses protected by Copyright Law, contact the copyright holder or the author.
dc.titleUltrastrong coupling of polar phonons and effective epsilon-near-zero modes in coaxial nanocavitiesen_US
dc.typeTexten_US

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