Assessment of dust size retrievals based on AERONET: A case study of radiative closure from visible-near-infrared to thermal infrared

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Abstract

Super-coarse dust particles (diameters > 10 µm) are evidenced to be more abundant in the atmosphere than model estimates and contribute significantly to the dust climate impacts. Since super-coarse dust accounts for less dust extinction in the visible-to-near-infrared (VIS-NIR) than in the thermal infrared (TIR) spectral regime, they are suspected to be underestimated by remote sensing instruments operates only in VIS-NIR, including Aerosol Robotic Networks (AERONET), a widely used dataset for dust model validation. In this study, we perform a radiative closure assessment using the AERONET-retrieved size distribution in comparison with the collocated Atmospheric Infrared Sounder (AIRS) TIR observations with comprehensive uncertainty analysis. The consistently warm bias in the comparisons suggests a potential underestimation of supercoarse dust in the AERONET retrievals due to the limited VIS-NIR sensitivity. An extra super coarse mode included in the AERONET-retrieved size distribution helps improve the TIR closure without deteriorating the retrieval accuracy in the VIS-NIR.